Theory of time- and frequency-gated spontaneous emission from systems with nonadiabatic coupling and dissipation [Elektronische Ressource] / Andrei Pisliakov

dieInstitutDomcf?rnat.)PheiysikGradesaliscT?rlerheLaubundM?ncTheoretiscdesheNaturwissenscChemie,orsitzender:Lehrstuhl1.f?rUniv.-Prof.TheoretiscwurdehehniscChemietderChemieTademiscecDoktorshnisc(Dr.henDissertation.UnivDr.ersit?tderM?ncDr.heneTheoryh.c.ofDietime-8.10.2003andTfrequency-gatedUnivspeingereicondurctaneousakult?temission4.11.2003fromaksystemshenwitheinesnonadiabaticdercouplinghaftenandrer.dissipationgenehmigtenAndreiVPisliakUniv.-Prof.oA.vPr?ferVDissertation:ollst?ndigerUniv.-Prof.AbW.druckk2.derDr.vA.onerauderDissertationFamakult?tbf?rderChemieecderhenTersit?techenhnischhenundUnivhersit?tFM?ncf?rhenamzurangenommen.Erlangung.Con.ten.ts.1.In.tro.duction.1.23.4Time-.and36frequency-gated.sp.on.taneous3.2.2emission:.general.theory.7.2.1.In.tro.duction..4.2.40.4.2.2.....resp.....wnian...3.3.1.......................transfer...............25....7.2.2.Denition.of.the.time-resolvresolutioned.sp.ectrum........functions.....eects...............Analytic....9342.3.P.olarization..3.5.........uorescence.In.........del...............(Redeld...42.Harmonic...............3.2.1.functions..11.2.3.1.Denition....and.........3.3.................resp...........3.3.2...............oscillator11.2.3.2.Calculation.of.the.p.olarization:.p33erturbativonsee.approac.h......Memory....13.2.3.3.Time-.and.frequency-resolv.ed.signal.in.terms.of.resp.onse.functions.15.2.3.4Time-resolvCalculationultrafastof39respductiononse.functions..............transfer...............Hamiltonians....16.2.4.